Revision of the World Meteorological Organization Global Atmosphere Watch (WMO/GAW) CO2 calibration scale Atmospheric Measurement Techniques DOI 10.5194/amt-14-3015-2021 16 June 2021 We have recently revised the carbon dioxide calibration scale used by numerous laboratories that measure atmospheric CO2. The revision follows from an improved understanding of the manometric method used to determine the absolute amount of CO2 in an atmospheric air sample. The new scale is 0.18 μmol mol−1 (ppm) greater than the previous scale at 400 ppm CO2. While this difference is small in relative terms (0.045 %), it is significant in terms of atmospheric monitoring. Read more
Observing the timescales of aerosol–cloud interactions in snapshot satellite images Atmospheric Chemistry and Physics DOI 10.5194/acp-21-6093-2021 15 June 2021 Cloud responses to aerosol are time-sensitive, but this development is rarely observed. This study uses isolated aerosol perturbations from ships to measure this development and shows that macrophysical (width, cloud fraction, detectability) and microphysical (droplet number) properties of ship tracks vary strongly with time since emission, background cloud and meteorological state. This temporal development should be considered when constraining aerosol–cloud interactions with observations. Read more
On the attribution of industrial-era glacier mass loss to anthropogenic climate change The Cryosphere DOI 10.5194/tc-15-1889-2021 14 June 2021 The worldwide retreat of mountain glaciers and consequent loss of ice mass is one of the most obvious signs of a changing climate and has significant implications for the hydrology and natural hazards in mountain landscapes. Consistent with our understanding of the human role in temperature change, we demonstrate that the central estimate of the size of the human-caused mass loss is essentially 100 % of the observed loss. This assessment resolves some important inconsistencies in the literature. Read more
Development of smart boulders to monitor mass movements via the Internet of Things: a pilot study in Nepal Earth Surface Dynamics DOI 10.5194/esurf-9-295-2021 11 June 2021 We use long-range smart sensors connected to a network based on the Internet of Things to explore the possibility of detecting hazardous boulder movements in real time. Prior to the 2019 monsoon season we inserted the devices in 23 boulders spread over debris flow channels and a landslide in northeastern Nepal. The data obtained in this pilot study show the potential of this technology to be used in remote hazard-prone areas in future early warning systems. Read more
Robust increase of Indian monsoon rainfall and its variability under future warming in CMIP6 models Earth System Dynamics DOI 10.5194/esd-12-367-2021 10 June 2021 All state-of-the-art global climate models that contributed to the latest Coupled Model Intercomparison Project (CMIP6) show a robust increase in Indian summer monsoon rainfall that is even stronger than in the previous intercomparison (CMIP5). Furthermore, they show an increase in the year-to-year variability of this seasonal rainfall that crucially influences the livelihood of more than 1 billion people in India. Read more
Uncertainties in the Emissions Database for Global Atmospheric Research (EDGAR) emission inventory of greenhouse gases Atmospheric Chemistry and Physics DOI 10.5194/acp-21-5655-2021 10 June 2021 We conducted an extensive analysis of the structural uncertainty of the Emissions Database for Global Atmospheric Research (EDGAR) emission inventory of greenhouse gases, which adds a much needed reliability dimension to the accuracy of the emission estimates. The study undertakes in-depth analyses of the implication of aggregating emissions from different sources and/or countries on the accuracy. Results are presented for all emissions sectors according to IPCC definitions. Read more
Snapshots of mean ocean temperature over the last 700 000 years using noble gases in the EPICA Dome C ice core Climate of the Past DOI 10.5194/cp-17-843-2021 9 June 2021 Using the temperature-dependent solubility of noble gases in ocean water, we reconstruct global mean ocean temperature (MOT) over the last 700 kyr using noble gas ratios in air enclosed in polar ice cores. Our record shows that glacial MOT was about 3 °C cooler compared to the Holocene. Interglacials before 450 kyr ago were characterized by about 1.5 °C lower MOT than the Holocene. In addition, some interglacials show transient maxima in ocean temperature related to changes in ocean circulation. Read more
Pervasive diffusion of climate signals recorded in ice-vein ionic impurities The Cryosphere DOI 10.5194/tc-15-1787-2021 8 June 2021 Current theory predicts climate signals in the vein chemistry of ice cores to migrate, hampering their dating. I show that the Gibbs–Thomson effect, which has been overlooked, causes fast diffusion that prevents signals from surviving into deep ice. Hence the deep climatic peaks in Antarctic and Greenlandic ice must be due to impurities in the ice matrix (outside veins) and safe from migration. These findings reset our understanding of postdepositional changes of ice-core climate signals. Read more
FES2014 global ocean tide atlas: design and performance Ocean Science DOI 10.5194/os-17-615-2021 7 June 2021 Since the mid-1990s, a series of FES (finite element solution) global ocean tidal atlases has been produced with the primary objective to provide altimetry missions with a tidal de-aliasing correction. We describe the underlying hydrodynamic/data assimilation design and accuracy assessments for the FES2014 release. The FES2014 atlas shows overall improved performance and has consequently been integrated in satellite altimetry and gravimetric data processing and adopted in ITRF standards. Read more
A Dark Target research aerosol algorithm for MODIS observations over eastern China: increasing coverage while maintaining accuracy at high aerosol loading Atmospheric Measurement Techniques DOI 10.5194/amt-14-3449-2021 7 June 2021 Due to fast industrialization and development, China has been experiencing haze pollution episodes with both high frequencies and severity over the last 3 decades. This study improves the accuracy and data coverage of measured aerosol from satellites, which help quantify, characterize, and understand the impact of the haze phenomena over the entire East Asia region. Read more
Introducing hydrometeor orientation into all-sky microwave and submillimeter assimilation Atmospheric Measurement Techniques DOI 10.5194/amt-14-3427-2021 4 June 2021 Oriented nonspherical ice particles induce polarization that is ignored when cloud-sensitive satellite observations are used in numerical weather prediction systems. We present a simple approach for approximating particle orientation, requiring minor adaption of software and no additional calculation burden. With this approach, the system realistically simulates the observed polarization patterns, increasing the physical consistency between instruments with different polarizations. Read more
Captured cirrus ice particles in high definition Atmospheric Chemistry and Physics DOI 10.5194/acp-21-7171-2021 2 June 2021 The cryo-electron microscopy images and analysis in this paper result from the first balloon-borne capture, preservation, and high-resolution imaging of ice particles from cirrus clouds. The images show cirrus particle complexity in unprecedented detail, revealing unexpected morphology, a mixture of surface roughness scales and patterns, embedded aerosols, and a large variety of habits within a single cloud. The results should inform ongoing efforts to refine modeling of cirrus radiative impact. Read more
High-frequency monitoring of anomalous methane point sources with multispectral Sentinel-2 satellite observations Atmospheric Measurement Techniques DOI 10.5194/amt-14-2771-2021 31 May 2021 Satellites can detect methane emissions by measuring sunlight reflected from the Earth’s surface and atmosphere. Here we show that the European Space Agency’s Sentinel-2 twin satellites can be used to monitor anomalously large methane point sources around the world, with global coverage every 2–5 days and 20 m spatial resolution. We demonstrate this previously unreported capability through high-frequency Sentinel-2 monitoring of two strong methane point sources in Algeria and Turkmenistan. Read more
JlBox v1.1: a Julia-based multi-phase atmospheric chemistry box model Geoscientific Model Development DOI 10.5194/gmd-14-2187-2021 28 May 2021 As our knowledge and understanding of atmospheric aerosol particle evolution and impact grows, designing community mechanistic models requires an ability to capture increasing chemical, physical and therefore numerical complexity. As the landscape of computing software and hardware evolves, it is important to profile the usefulness of emerging platforms in tackling this complexity. With this in mind we present JlBox v1.1, written in Julia. Read more
Sudden large-volume detachments of low-angle mountain glaciers – more frequent than thought? The Cryosphere DOI 10.5194/tc-15-1751-2021 26 May 2021 Hardly recognized so far, giant catastrophic detachments of glaciers are a rare but great potential for loss of lives and massive damage in mountain regions. Several of the events compiled in our study involve volumes (up to 100 million m3 and more), avalanche speeds (up to 300 km/h), and reaches (tens of kilometres) that are hard to imagine. We show that current climate change is able to enhance associated hazards. For the first time, we elaborate a set of factors that could cause these events. Read more
African easterly waves in an idealized general circulation model: instability and wave packet diagnostics Weather and Climate Dynamics DOI 10.5194/wcd-2-311-2021 24 May 2021 Using a simple general circulation model, we examine the structure of waves in the mid-tropospheric jet over North Africa. We show that waves occur in near-stationary groups or wave packets. As they are not swept out of the jet, this may provide the opportunity for the packets to amplify via feedback from other energy sources like rain-producing cloud complexes and mineral dust that are known to operate here. Our results address the criticism that the easterly jet is too short to sustain waves. Read more
Medusa–Aqua system: simultaneous measurement and evaluation of novel potential halogenated transient tracers HCFCs, HFCs, and PFCs in the ocean Ocean Science DOI 10.5194/os-17-509-2021 21 May 2021 Observations of transient tracer distribution provide essential information on ocean ventilation. The use of several commonly used transient traces is limited as their atmospheric mole fractions do not monotonically change. Here we explore new potential oceanic transient tracers with an analytical system that simultaneously measures a large range of compounds. Combined with the known atmospheric history and seawater solubility, we discuss the utility of selected HCFCs, HFCs, and PFCs as tracers. Read more
Summary and synthesis of Changing Cold Regions Network (CCRN) research in the interior of western Canada – Part 2: Future change in cryosphere, vegetation, and hydrology Hydrology and Earth System Sciences DOI 10.5194/hess-25-1849-2021 19 May 2021 This article examines future changes in land cover and hydrological cycling across the interior of western Canada under climate conditions projected for the 21st century. Key insights into the mechanisms and interactions of Earth system and hydrological process responses are presented, and this understanding is used together with model application to provide a synthesis of future change. This has allowed more scientifically informed projections than have hitherto been available. Read more
Arctic Ocean acidification over the 21st century co-driven by anthropogenic carbon increases and freshening in the CMIP6 model ensemble Biogeosciences DOI 10.5194/bg-18-2221-2021 17 May 2021 The uptake of carbon, emitted as a result of human activities, results in ocean acidification. We analyse 21st-century projections of acidification in the Arctic Ocean, a region of particular vulnerability, using the latest generation of Earth system models. In this new generation of models there is a large decrease in the uncertainty associated with projections of Arctic Ocean acidification, with freshening playing a greater role in driving acidification than previously simulated. Read more
Airborne measurements of oxygen concentration from the surface to the lower stratosphere and pole to pole Atmospheric Measurement Techniques DOI 10.5194/amt-14-2543-2021 14 May 2021 We describe methods used to make high-precision global-scale airborne measurements of atmospheric oxygen concentrations over a period of 20 years in order to study the global carbon cycle. Our techniques include an in situ vacuum ultraviolet absorption instrument and a pressure- and flow-controlled, cryogenically dried, glass flask sampler. We have deployed these instruments in 15 airborne research campaigns spanning from the Earth’s surface to the lower stratosphere and from pole to pole. Read more