Agricultural ammonia emissions in China: reconciling bottom-up and top-down estimates Atmospheric Chemistry and Physics DOI 10.5194/acp-18-339-2018 12 January 2018 Substantial differences exist in current estimates of agricultural ammonia emissions in China, hindering understanding of their environmental consequences. This study applies both bottom-up and top-down methods to better quantify agricultural ammonia sources in China using observations from satellite and surface networks interpreted by a chemical transport model. Our estimate of annual Chinese anthropogenic ammonia emission is 11.7 tg (teragram) for 2008 with a strong seasonality peak in summer. Read more
Temporal variability of tidal and gravity waves during a record long 10-day continuous lidar sounding Atmospheric Chemistry and Physics DOI 10.5194/acp-18-371-2018 12 January 2018 Gravity waves (GWs) as well as solar tides are a key driving mechanism for the circulation in the Earth’s atmosphere. The temporal variation of these waves is studied using a record long 10-day continuous Rayleigh–Mie–Raman lidar sounding at midlatitudes. This data set shows a large variability of these waves on timescales of a few days and therefore provides new insights into wave intermittency phenomena, which can help to improve model simulations. Read more
First tomographic observations of gravity waves by the infrared limb imager GLORIA Atmospheric Chemistry and Physics DOI 10.5194/acp-17-14937-2017 18 December 2017 Using the infrared limb imager GLORIA, the 3-D structure of mesoscale gravity waves in the lower stratosphere was measured for the first time, allowing for a complete 3-D characterization of the waves. This enables the precise determination of the sources of the waves in the mountain regions of Iceland with backward ray tracing. Forward ray tracing shows oblique propagation, an effect generally neglected in global atmospheric models. GLORIA">Read more
The role of meteorological conditions and pollution control strategies in reducing air pollution in Beijing during APEC 2014 and Victory Parade 2015 Atmospheric Chemistry and Physics DOI 10.5194/acp-17-13921-2017 23 November 2017 The generalized linear regression model (GLM), even based only on meteorological parameters, could be satisfactory to estimate the contribution of meteorological conditions in reducing air pollution and hence the contribution of control strategies in reducing air pollution. Using the GLM, we found that the meteorological conditions and pollution control strategies contributed 30% and 28% to the reduction of the PM2.5 concentration during APEC 2014 and 38% and 25% during Parade 2015. APEC 2014 and Victory Parade 2015">Read more
A new diagnostic for tropospheric ozone production Atmospheric Chemistry and Physics DOI 10.5194/acp-17-13669-2017 17 November 2017 Understanding tropospheric ozone chemistry has been at the centre of the field of atmospheric chemistry for the last 30 years. However, our conceptual approach to diagnosing ozone production in global models has not advanced in this time. Our work presents a new and powerful approach for diagnosing tropospheric ozone production, providing a significant enhancement in our ability to understand the processes controlling ozone and how we can validate our assessment of these processes. Read more
Impact of agricultural emission reductions on fine-particulate matter and public health Atmospheric Chemistry and Physics DOI 10.5194/acp-17-12813-2017 27 October 2017 This study shows that agricultural emissions are important for air quality and their reduction can effectively reduce the concentration of fine particles and their associated premature mortality. Therefore, emission control policies, especially in North America and Europe, should also involve strong ammonia emission decreases to optimally reduce fine-particle concentration. Read more
A growing threat to the ozone layer from short-lived anthropogenic chlorocarbons Atmospheric Chemistry and Physics DOI 10.5194/acp-17-11929-2017 12 October 2017 We have observed large amounts of man-made chlorine compounds in E and SE Asia and in the upper tropical troposphere. These relatively short-lived compounds are not controlled by the Montreal Protocol, but if significant quantities were able to reach the stratosphere, the long-term recovery of stratospheric ozone would be delayed. We have also identified an important atmospheric transport mechanism that can rapidly transport these chemicals from E Asia to the upper troposphere via the tropics. Read more
An update on ozone profile trends for the period 2000 to 2016 Atmospheric Chemistry and Physics DOI 10.5194/acp-17-10675-2017 11 September 2017 Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000. Read more
Simultaneous measurements of new particle formation at 1 s time resolution at a street site and a rooftop site Atmospheric Chemistry and Physics DOI 10.5194/acp-17-9469-2017 8 August 2017 This study reports the distinct effects of street canyons on new particle formation (NPF) under warm or cold ambient temperature conditions because of on-road vehicle emissions; i.e., stronger condensation sinks are responsible for the reduced NPF in the springtime, but efficient nucleation and partitioning of gaseous species contribute to the enhanced NPF in the wintertime. The oxidization of biogenic organics is suggested to play an important role in growing new particles. Read more
NOx emission trends over Chinese cities estimated from OMI observations during 2005 to 2015 Atmospheric Chemistry and Physics DOI 10.5194/acp-17-9261-2017 1 August 2017 We assess NOx emission trends over Chinese cities based on satellite NO2 observations using a method independent of chemical transport models. NOx emissions over 48 Chinese cities have decreased significantly since 2011. Cities with different dominant emission sources (i.e. power, industrial, and transportation sectors) showed variable emission decline timelines that corresponded to the schedules for emission control in different sectors. OMI observations during 2005 to 2015">Read more