A tropical West Pacific OH minimum and implications for stratospheric composition Atmospheric Chemistry and Physics DOI 10.5194/acp-14-4827-2014 15 May 2014 Most of the short-lived biogenic and anthropogenic chemical species that are emitted into the atmosphere break down efficiently by reaction with OH and do not reach the stratosphere. Here we show the existence of a pronounced minimum in the tropospheric column of ozone over the West Pacific, the main source region for stratospheric air, and suggest a corresponding minimum of the tropospheric column of OH. Read more
Effects of stratospheric ozone recovery on photochemistry and ozone air quality in the troposphere Atmospheric Chemistry and Physics DOI 10.5194/acp-14-4079-2014 23 April 2014 In this study, the authors examine the implications of stratospheric ozone recovery for the tropospheric chemistry and ozone air quality with a global chemical transport model (GEOS-Chem). Read more
Further evidence of important environmental information content in red-to-green ratios as depicted in paintings by great masters Atmospheric Chemistry and Physics DOI 10.5194/acp-14-2987-2014 25 March 2014 In this paper, the authors examine sunsets painted by famous artists as proxy information for the aerosol optical depth after major volcanic eruptions. Read more
Characterization of submicron aerosols during a month of serious pollution in Beijing, 2013 Atmospheric Chemistry and Physics DOI 10.5194/acp-14-2887-2014 20 March 2014 In January 2013, Beijing experienced several serious haze events. To achieve a better understanding of the characteristics, sources and processes of aerosols during this month, an Aerodyne high-resolution time-of-flight aerosol mass spectrometer was deployed at an urban site between 1 January and 1 February 2013 to obtain the size-resolved chemical composition of non-refractory submicron particles. Read more
Uncertainty analysis of projections of ozone-depleting substances: mixing ratios, EESC, ODPs, and GWPs Atmospheric Chemistry and Physics DOI 10.5194/acp-14-2757-2014 17 March 2014 Here the authors present a comprehensive uncertainty analysis of future mixing ratios of ozone-depleting substances (ODPs), levels of equivalent effective stratospheric chlorine (EESC), ozone depletion potentials, and global warming potentials (GWPs). EESC, ODPs, and GWPs">Read more
Incidence of rough and irregular atmospheric ice particles from Small Ice Detector 3 measurements Atmospheric Chemistry and Physics DOI 10.5194/acp-14-1649-2014 12 February 2014 2D light-scattering patterns were obtained in situ for the first time using the Small Ice Detector 3 probe during several flights in a variety of mid-latitude mixed-phase and cirrus clouds. Read more
Microphysical properties and high ice water content in continental and oceanic mesoscale convective systems and potential implications for commercial aircraft at flight altitude Atmospheric Chemistry and Physics DOI 10.5194/acp-14-899-2014 27 January 2014 Two complementary case studies are conducted to analyse convective system properties in the region where strong cloud-top lidar backscatter anomalies are observed as reported by Platt et al. (2011). Read more
Arctic stratospheric dehydration – Part 1: Unprecedented observation of vertical redistribution of water Atmospheric Chemistry and Physics DOI 10.5194/acp-13-11503-2013 27 November 2013 This paper presents high-resolution measurements of water vapour, aerosols and clouds in the Arctic stratosphere in January and February 2010 carried out by in situ instrumentation on balloon sondes and high-altitude aircraft combined with satellite observations. Read more
Quantifying aerosol mixing state with entropy and diversity measures Atmospheric Chemistry and Physics DOI 10.5194/acp-13-11423-2013 25 November 2013 This paper presents the first quantitative metric for aerosol population mixing state, defined as the distribution of per-particle chemical species composition. Read more
Heterogeneous formation of polar stratospheric clouds – Part 2: Nucleation of ice on synoptic scales Atmospheric Chemistry and Physics DOI 10.5194/acp-13-10769-2013 6 November 2013 This paper provides compelling evidence for the importance of heterogeneous nucleation, likely on solid particles of meteoritic origin, and of small-scale temperature fluctuations, for the formation of ice particles in the Arctic stratosphere. Read more