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Molecular simulations reveal that heterogeneous ice nucleation occurs at higher temperatures in water under capillary tension

Using computer simulations of water, we find that water under tension freezes more easily than under normal conditions. A linear equation describes how freezing temperature increases with tension. Accordingly, simulations show that naturally occurring tension in water capillary bridges leads to higher freezing temperatures. This work is an early step in determining if atmospheric cloud droplets freeze due to naturally occurring tension, for example, during processes such as droplet collisions.

Opinion: Atmospheric multiphase chemistry – past, present, and future

With important climate and air quality impacts, atmospheric multiphase chemistry involves gas interactions with aerosol particles and cloud droplets. We summarize the status of the field and discuss potential directions for future growth. We highlight the importance of a molecular-level understanding of the chemistry, along with atmospheric field studies and modelling, and emphasize the necessity for atmospheric multiphase chemists to interact widely with scientists from neighbouring disciplines.

Atmospheric CO2 inversion reveals the Amazon as a minor carbon source caused by fire emissions, with forest uptake offsetting about half of these emissions

The Amazon’s carbon balance may have changed due to forest degradation, deforestation and warmer climate. We used an atmospheric model and atmospheric CO2 observations to quantify Amazonian carbon emissions (2010–2018). The region was a small carbon source to the atmosphere, mostly due to fire emissions. Forest uptake compensated for ~ 50 % of the fire emissions, meaning that the remaining forest is still a small carbon sink. We found no clear evidence of weakening carbon uptake over the period.

A rise in HFC-23 emissions from eastern Asia since 2015

Based on atmospheric HFC-23 observations, the first estimate of post-CDM HFC-23 emissions in eastern Asia for 2008-2019 shows that these emissions contribute significantly to the global emissions rise. The observation-derived emissions were much larger than the bottom-up estimates expected to approach zero after 2015 due to national abatement activities. These discrepancies could be attributed to unsuccessful factory-level HFC-23 abatement and inaccurate quantification of emission reductions.

HFC-23 emissions from eastern Asia since 2015">Read more

Detection of large-scale cloud microphysical changes within a major shipping corridor after implementation of the International Maritime Organization 2020 fuel sulfur regulations

Fuel sulfur regulations were implemented for ships in 2020 to improve air quality but may also accelerate global warming. We use spatial statistics and satellite retrievals to detect changes in the size of cloud droplets and find evidence for a resulting decrease in cloud brightness within a major shipping corridor after the sulfur limits went into effect. Our results confirm both that the regulations are being followed and that they are having a warming influence via their effect on clouds.

Continuous weekly monitoring of methane emissions from the Permian Basin by inversion of TROPOMI satellite observations

We use TROPOMI satellite observations to quantify weekly methane emissions from the US Permian oil and gas basin from May 2018 to October 2020. We find that Permian emissions are highly variable, with diverse economic and activity drivers. The most important drivers during our study period were new well development and natural gas price. Permian methane intensity averaged 4.6% and decreased by 1% per year.

TROPOMI satellite observations">Read more

Impact of a strong volcanic eruption on the summer middle atmosphere in UA-ICON simulations

Strong volcanic eruptions are able to alter the temperature and the circulation of the middle atmosphere. This study simulates the atmospheric response to an idealized strong tropical eruption and focuses on the impact on the mesosphere. The simulations show a warming of the polar summer mesopause in the first November after the eruption. Our study indicates that this is mainly due to dynamical coupling in the summer hemisphere with a potential contribution from interhemispheric coupling.

ICON simulations">Read more

Particle shapes and infrared extinction spectra of nitric acid dihydrate (NAD) crystals: optical constants of the β-NAD modification

Polar stratospheric clouds (PSCs) play an important role in the depletion of stratospheric ozone. They can consist of different chemical species, including crystalline nitric acid hydrates. We found that mineral dust or meteoric ablation material can efficiently catalyse the formation of a specific phase of nitric acid dihydrate crystals. We determined predominant particle shapes and infrared optical properties of these crystals, which are important inputs for remote sensing detection of PSCs.

NAD) crystals: optical constants of the β-NAD modification">Read more

Opinion: How fear of nuclear winter has helped save the world, so far

A nuclear war could produce a nuclear winter, with catastrophic consequences for global food supplies. Nuclear winter theory helped to end the nuclear arms race in the 1980s, but more than 10,000 nuclear weapons still exist. This means they can be used, by unstable leaders, accidentally from technical malfunctions or human error, or by terrorists. Therefore, it is urgent for scientists to study these issues, broadly communicate their results, and work for the elimination of nuclear weapons.

Opinion: The scientific and community-building roles of the Geoengineering Model Intercomparison Project (GeoMIP) – past, present, and future

Geoengineering indicates methods aiming to reduce the temperature of the planet by means of reflecting back a part of the incoming radiation before it reaches the surface or allowing more of the planetary radiation to escape into space. It aims to produce modelling experiments that are easy to reproduce and compare with different climate models, in order to understand the potential impacts of these techniques. Here we assess its past successes and failures and talk about its future.

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