Stratospheric residence time and the lifetime of volcanic stratospheric aerosols Atmospheric Chemistry and Physics DOI 10.5194/acp-25-3821-2025 4 April 2025 The climate impact of volcanic eruptions depends in part on how long aerosols spend in the stratosphere. We develop a conceptual model for stratospheric aerosol lifetime in terms of production and decay timescales, as well as a lag between injection and decay. We find residence time depends strongly on injection height in the lower stratosphere. We show that the lifetime of stratospheric aerosol from the 1991 Pinatubo eruption is around 22 months, significantly longer than is commonly reported. Read more
Pristine oceans are a significant source of uncertainty in quantifying global cloud condensation nuclei Atmospheric Chemistry and Physics DOI 10.5194/acp-25-3841-2025 2 April 2025 Aerosol particles in the atmosphere increase cloud reflectivity, thereby cooling the Earth. Accurate global measurements of these particles are crucial for estimating this cooling effect. This study compares and harmonizes two newly developed global aerosol datasets, offering insights for their future use and refinement. We identify pristine oceans as a significant source of uncertainty in the datasets and, therefore, in quantifying the role of aerosols in Earth's climate. Read more
Modulation of the northern polar vortex by the Hunga Tonga–Hunga Ha'apai eruption and the associated surface response Atmospheric Chemistry and Physics DOI 10.5194/acp-25-3623-2025 28 March 2025 In January 2022, the Hunga Tonga–Hunga Ha'apai (HTHH) volcano erupted, sending massive amounts of water vapour into the atmosphere. This event had a significant impact on stratospheric and lower-mesospheric chemical composition. Two years later, stratospheric conditions were disturbed during so-called sudden stratospheric warmings. Here we simulate a novel pathway by which this water-rich eruption may have contributed to conditions during these events and consequently impacted the surface climate. Read more
Modelled surface climate response to effusive Icelandic volcanic eruptions: sensitivity to season and size Atmospheric Chemistry and Physics DOI 10.5194/acp-25-2989-2025 19 March 2025 We use an Earth system model to systematically investigate the climate response to high-latitude effusive volcanic eruptions as a function of eruption season and size, with a focus on the Arctic. We find that different seasons strongly modulate the climate response, with Arctic surface warming observed in winter and cooling in summer. Additionally, as eruptions increase in terms of sulfur dioxide emissions, the climate response becomes increasingly insensitive to variations in emission strength. Read more
Opinion: Why all emergent constraints are wrong but some are useful – a machine learning perspective Atmospheric Chemistry and Physics DOI 10.5194/acp-25-2365-2025 26 February 2025 In our article, we review uncertainties in global climate change projections and current methods using Earth observations as constraints, which is crucial for climate risk assessments and for informing society. We then discuss how machine learning can advance the field, discussing recent work that provides potentially stronger and more robust links between observed data and future climate projections. We further discuss the challenges of applying machine learning to climate science. Read more
Opinion: Understanding the impacts of agriculture and food systems on atmospheric chemistry is instrumental to achieving multiple Sustainable Development Goals Atmospheric Chemistry and Physics DOI 10.5194/acp-25-923-2025 28 January 2025 We discuss our current understanding of and knowledge gaps in how agriculture and food systems affect air quality and how agricultural emissions can be mitigated. We argue that scientists need to address these gaps, especially as the importance of fossil fuel emissions is fading. This will help guide food-system transformation in economically viable, socially inclusive, and environmentally responsible ways and is essential to help society achieve sustainable development. Read more
Warming effects of reduced sulfur emissions from shipping Atmospheric Chemistry and Physics DOI 10.5194/acp-24-13681-2024 24 December 2024 A 2020 regulation has reduced sulfur emissions from shipping by about 80 %, leading to a decrease in atmospheric aerosols that have a cooling effect primarily by affecting cloud properties and amounts. Our climate model simulations predict a global temperature increase of 0.04 K over the next 3 decades as a result, which could contribute to surpassing the Paris Agreement’s 1.5 °C target. Reduced aerosols may have also contributed to the recent temperature spikes. Read more
Lidar measurements of noctilucent clouds at Río Grande, Tierra del Fuego, Argentina Atmospheric Chemistry and Physics DOI 10.5194/acp-24-14029-2024 17 December 2024 Noctilucent clouds (NLCs) are silvery clouds that can be viewed during twilight and indicate atmospheric conditions like temperature and water vapor in the upper mesosphere. High-resolution measurements from a remote sensing laser instrument provide NLC height, brightness, and occurrence rate since 2017. Most observations occur in the morning hours, likely caused by strong tidal winds, and NLC ice particles are thus transported from elsewhere to the observing location in the Southern Hemisphere. Read more
Opinion: Challenges and needs of tropospheric chemical mechanism development Atmospheric Chemistry and Physics DOI 10.5194/acp-24-13317-2024 9 December 2024 Chemical mechanisms describe the chemical processes in atmospheric models that are used to describe the changes in the atmospheric composition. Therefore, accurate chemical mechanisms are necessary to predict the evolution of air pollution and climate change. The article describes all steps that are needed to build chemical mechanisms and discusses the advances and needs of experimental and theoretical research activities needed to build reliable chemical mechanisms. Read more
Weak liquid water path response in ship tracks Atmospheric Chemistry and Physics DOI 10.5194/acp-24-13269-2024 5 December 2024 Ship emissions can form artificially brightened clouds, known as ship tracks, and provide us with an opportunity to investigate how aerosols interact with clouds. Previous studies that used ship tracks suggest that clouds can experience large increases in the amount of water (LWP) from aerosols. Here, we show that there is a bias in previous research and that, when we account for this bias, the LWP response to aerosols is much weaker than previously reported. Read more