Opinion: The role of AerChemMIP in advancing climate and air quality research Atmospheric Chemistry and Physics DOI 10.5194/acp-25-8289-2025 31 July 2025 The Aerosol Chemistry Model Intercomparison Project (AerChemMIP) aimed to quantify the climate and air quality impacts of aerosols and chemically reactive gases. We review its contribution to AR6 (Sixth Assessment Report of the Intergovernmental Panel on Climate Change) and the wider understanding of the role of these species in climate and climate change. We identify challenges and provide recommendations to improve the utility and uptake of climate model data, detailed summary tables of CMIP6 models, experiments, and emergent diagnostics. Read more
Observational constraints suggest a smaller effective radiative forcing from aerosol–cloud interactions Atmospheric Chemistry and Physics DOI 10.5194/acp-25-7299-2025 17 July 2025 This study addresses the long-standing challenge of quantifying the impact of aerosol–cloud interactions. Using satellite observations, reanalysis data, and a "perfect-model" cross-validation, we show that explicitly accounting for aerosol–cloud droplet activation rates is key to accurately estimating ERFaci (effective radiative forcing due to aerosol–cloud interactions). Our results indicate a smaller and less uncertain ERFaci than previously assessed, implying the reduced role of aerosol–cloud interactions in shaping climate sensitivity. Read more
Implications of reduced-complexity aerosol thermodynamics on organic aerosol mass concentration and composition over North America Atmospheric Chemistry and Physics DOI 10.5194/acp-25-5773-2025 12 June 2025 We implemented the BAT-VBS (Binary Activity Thermodynamics volatility basis set) aerosol thermodynamics model in the GEOS-Chem chemical transport model to efficiently account for organic aerosol water uptake, nonideal mixing, and impacts on the gas–particle partitioning of semi-volatile organics. Compared to GEOS-Chem's complex (dry) scheme, we show that the BAT-VBS model can predict substantial enhancements in organic aerosol mass concentration at moderate-to-high relative humidity. Read more
Explaining the period fluctuation of the quasi-biennial oscillation Atmospheric Chemistry and Physics DOI 10.5194/acp-25-5647-2025 6 June 2025 The paper addresses a fundamental but unresolved question about the tropical stratospheric wind oscillation: why does the period of the oscillation fluctuate irregularly? We use global reanalysis data to provide evidence that the oscillation period is primarily modulated by seasonal variations in small-scale atmospheric wave activity. The findings have implications for seasonal and climate predictions. Read more
Quantified ice-nucleating ability of AgI-containing seeding particles in natural clouds Atmospheric Chemistry and Physics DOI 10.5194/acp-25-5387-2025 2 June 2025 We analyzed the ability of silver iodide particles (a commonly used cloud-seeding agent) to form ice crystals in naturally occurring liquid clouds at −5 to −8 °C and found that only ≈ 0.1 %−1 % of particles nucleate ice, with a negative dependence on temperature. By contextualizing our results with previous laboratory studies, we help to bridge the gap between laboratory and field experiments, which also helps to inform future cloud-seeding projects. Read more
Stratospheric residence time and the lifetime of volcanic stratospheric aerosols Atmospheric Chemistry and Physics DOI 10.5194/acp-25-3821-2025 4 April 2025 The climate impact of volcanic eruptions depends in part on how long aerosols spend in the stratosphere. We develop a conceptual model for stratospheric aerosol lifetime in terms of production and decay timescales, as well as a lag between injection and decay. We find residence time depends strongly on injection height in the lower stratosphere. We show that the lifetime of stratospheric aerosol from the 1991 Pinatubo eruption is around 22 months, significantly longer than is commonly reported. Read more
Pristine oceans are a significant source of uncertainty in quantifying global cloud condensation nuclei Atmospheric Chemistry and Physics DOI 10.5194/acp-25-3841-2025 2 April 2025 Aerosol particles in the atmosphere increase cloud reflectivity, thereby cooling the Earth. Accurate global measurements of these particles are crucial for estimating this cooling effect. This study compares and harmonizes two newly developed global aerosol datasets, offering insights for their future use and refinement. We identify pristine oceans as a significant source of uncertainty in the datasets and, therefore, in quantifying the role of aerosols in Earth's climate. Read more
Modulation of the northern polar vortex by the Hunga Tonga–Hunga Ha'apai eruption and the associated surface response Atmospheric Chemistry and Physics DOI 10.5194/acp-25-3623-2025 28 March 2025 In January 2022, the Hunga Tonga–Hunga Ha'apai (HTHH) volcano erupted, sending massive amounts of water vapour into the atmosphere. This event had a significant impact on stratospheric and lower-mesospheric chemical composition. Two years later, stratospheric conditions were disturbed during so-called sudden stratospheric warmings. Here we simulate a novel pathway by which this water-rich eruption may have contributed to conditions during these events and consequently impacted the surface climate. Read more
Modelled surface climate response to effusive Icelandic volcanic eruptions: sensitivity to season and size Atmospheric Chemistry and Physics DOI 10.5194/acp-25-2989-2025 19 March 2025 We use an Earth system model to systematically investigate the climate response to high-latitude effusive volcanic eruptions as a function of eruption season and size, with a focus on the Arctic. We find that different seasons strongly modulate the climate response, with Arctic surface warming observed in winter and cooling in summer. Additionally, as eruptions increase in terms of sulfur dioxide emissions, the climate response becomes increasingly insensitive to variations in emission strength. Read more
Opinion: Why all emergent constraints are wrong but some are useful – a machine learning perspective Atmospheric Chemistry and Physics DOI 10.5194/acp-25-2365-2025 26 February 2025 In our article, we review uncertainties in global climate change projections and current methods using Earth observations as constraints, which is crucial for climate risk assessments and for informing society. We then discuss how machine learning can advance the field, discussing recent work that provides potentially stronger and more robust links between observed data and future climate projections. We further discuss the challenges of applying machine learning to climate science. Read more