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Evaluation of global simulations of aerosol particle and cloud condensation nuclei number, with implications for cloud droplet formation

Effects of aerosols on clouds are important for climate studies but are among the largest uncertainties in climate projections. This study evaluates the skill of global models to simulate aerosol, cloud condensation nuclei (CCN) and cloud droplet number concentrations (CDNCs). Model results show reduced spread in CDNC compared to CCN due to the negative correlation between the sensitivities of CDNC to aerosol number concentration (air pollution) and updraft velocity (atmospheric dynamics).

Emission of trace gases and aerosols from biomass burning – an updated assessment

Biomass burning is one of the largest sources of atmospheric pollutants worldwide. This paper presents an up-to-date compilation of emission factors for over 120 trace gas and aerosol species from the different forms of open vegetation fires and domestic biofuel use, based on an analysis of over 370 published studies. Using these emission factors and current global burning activity data, the annual emissions of important species released by the various types of biomass burning are estimated.

Contrail cirrus radiative forcing for future air traffic

The climate impact of air traffic is to a large degree caused by changes in cirrus cloudiness resulting from the formation of contrails. We use an atmospheric climate model with a contrail cirrus parameterization to investigate the climate impact of contrail cirrus for the year 2050. The strong increase in contrail cirrus radiative forcing due to the projected increase in air traffic volume cannot be compensated for by the reduction of soot emissions and by improvements in propulsion efficiency.

Aerosol pH and its driving factors in Beijing

Aerosol acidity plays a key role in secondary aerosol formation. To provide a more comprehensive reference for aerosol pH and a basis for controlling secondary aerosol generation, this study used the latest data covering four seasons and different particle sizes to obtain the characteristics of aerosol pH and explore the main factors affecting aerosol pH and gas–particle partitioning in the Beijing area.

Global distribution of methane emissions, emission trends, and OH concentrations and trends inferred from an inversion of GOSAT satellite data for 2010–2015

We use 2010–2015 satellite observations of atmospheric methane to improve estimates of methane emissions and their trends, as well as the concentration and trend of tropospheric OH (hydroxyl radical, methane’s main sink). We find overestimates of Chinese coal and Middle East oil/gas emissions in the prior estimate. The 2010–2015 growth in methane is attributed to an increase in emissions from India, China, and areas with large tropical wetlands. The contribution from OH is small in comparison.

GOSAT satellite data for 2010–2015">Read more

Photooxidants from brown carbon and other chromophores in illuminated particle extracts

We measured hydroxyl radical (^•OH), singlet oxygen (¹O₂*), and organic triplets (³C*) in illuminated aqueous particle extracts. After measuring the impact of dilution on oxidant concentrations, we extrapolated our results to predict them in ambient particles –¹O₂* and³C* concentrations appear to be greatly enhanced, while^•OH appears largely unchanged. Two of these oxidants (¹O₂*,³C*) are not yet included in atmospheric models, and our results make it possible to include them in the future.

Northern Hemisphere continental winter warming following the 1991 Mt. Pinatubo eruption: reconciling models and observations

This study provides compelling new evidence that the surface winter warming observed over the Northern Hemisphere continents following the 1991 eruption of Mt. Pinatubo was, very likely, completely unrelated to the eruption. This result has implications for earlier eruptions, as the evidence presented here demonstrates that the surface signal of even the very largest known eruptions may be swamped by the internal variability at high latitudes.

Quantifying variations in shortwave aerosol–cloud–radiation interactions using local meteorology and cloud state constraints

Aerosols are released by natural and human activities. When aerosols encounter clouds they interact in what is known as the indirect effect. Brighter clouds are expected due to the microphysical response; however, certain environments can trigger a modified response. Limits on the stability, humidity, and cloud thickness are applied regionally to investigate local cloud responses to aerosol, resulting in a range of indirect effects that would result in significant cooling or slight warming.

Heterogeneous sulfate aerosol formation mechanisms during wintertime Chinese haze events: air quality model assessment using observations of sulfate oxygen isotopes in Beijing

Sulfate is a key species contributing to particle formation and growth during wintertime Chinese haze events. This study combines observations and modeling of oxygen isotope signatures in sulfate aerosol to investigate its formation mechanisms, with a focus on heterogeneous production on aerosol surface via H₂O₂, O₃, and NO₂ and trace metal catalyzed oxidation. Contributions from different formation pathways are presented.

Vertical and horizontal distribution of submicron aerosol chemical composition and physical characteristics across northern India during pre-monsoon and monsoon seasons

Our study, for the first time, presents measurements of aerosol chemical composition and physical characteristics across northern India in the pre-monsoon and monsoon seasons of 2016 using the FAAM BAe-146 UK research aircraft. Across northern India, an elevated aerosol layer dominated by sulfate aerosol exists that diminishes with monsoon arrival. The Indo-Gangetic Plain (IGP) boundary layer is dominated by organics, whereas outside the IGP sulfate dominates with increased scattering aerosol.

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