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Volatile organic compounds and ozone in Rocky Mountain National Park during FRAPPÉ

Rocky Mountain National Park experiences high ozone concentrations that can exceed the National Ambient Air Quality Standard. As part of the FRAPPÉ field campaign, a suite of volatile organic compounds were measured to characterize the sources of ozone precursors that contribute to high ozone in the park. These measurements indicate emissions from the Front Range in Colorado tied to oil and gas operations, urban areas, and the stratosphere contribute to episodes of elevated ozone.

FRAPPÉ">Read more

Structural changes in the shallow and transition branch of the Brewer–Dobson circulation induced by El Niño

This paper assesses the structural changes in the shallow and transition branches of the BDC induced by El Nino using the Lagrangian model simulations driven by ERAi and JRA-55 combined with MLS observations. We found a clear evidence of a weakening of the transition branch due to an upward shift in the dissipation height of the planetary and gravity waves and a strengthening of the shallow branch due to enhanced GW breaking in the tropics–subtropics and PW breaking at high latitudes.

Photochemical box modelling of volcanic SO2 oxidation: isotopic constraints

Volcanic sulfur can have climatic impacts for the planet via sulfate aerosol formation, leading also to pollution events. We provide model constraints on tropospheric volcanic sulfate formation, with implications for its lifetime and impacts on regional air quality. Oxygen isotope investigations from our model suggest that in the poor tropospheric plumes of halogens, the O2/TMI sulfur oxidation pathway might significantly control sulfate production. The produced sulfate has no isotopic anomaly.

The impact of mineral dust on cloud formation during the Saharan dust event in April 2014 over Europe

The impact of desert dust on cloud formation is investigated for a major Saharan dust event over Europe by interactive regional dust modeling. Dust particles are very efficient ice-nucleating particles promoting the formation of ice crystals in clouds. The simulations show that the observed extensive cirrus development was likely related to the above-average dust load. The interactive dust–cloud feedback in the model significantly improves the agreement with aircraft and satellite observations.

Mesospheric bores at southern midlatitudes observed by ISS-IMAP/VISI: a first report of an undulating wave front

Spatial structures of wave disturbances in the upper atmosphere were investigated with space-borne imaging from the International Space Station. The wave disturbance occurred around an altitude of 100 km, and is called a mesospheric bore. The large-scale structure of mesospheric bores has not been fully captured by previous ground-based imagers, but the space-borne imaging captured a bore with a wide field of view, and showed that bores can have a large undulating wave front as long as 2000 km.

ISS-IMAP/VISI: a first report of an undulating wave front">Read more

Additional global climate cooling by clouds due to ice crystal complexity

Using light diffraction it is possible to detect microscopic features within ice particles that have not yet been fully characterized. Here, this technique was applied in airborne measurements, where it was found that majority of atmospheric ice particles have features that significantly change the way ice particles interact with solar light. The microscopic features make ice-containing clouds more reflective than previously thought, which could have consequences for predicting our climate.

Mesoscale fine structure of a tropopause fold over mountains

GLORIA observations during two crossings of the polar front jet stream resolve the fine mesoscale structure of a tropopause fold in high detail. Tracer–tracer correlations of H₂O and O₃ are presented as a function of potential temperature and reveal an active mixing region. Our study confirms conceptual models of tropopause folds, validates the high quality of ECMWF IFS forecasts, and suggests that mountain waves are capable of modulating exchange processes in the vicinity of tropopause folds.

Ice crystal number concentration estimates from lidar–radar satellite remote sensing – Part 1: Method and evaluation

The number concentration of ice crystals (N_i) is a key cloud property that remains very uncertain due to difficulties in determining it using satellites. This lack of global observational constraints limits our ability to constrain this property in models responsible for predicting future climate. This pair of papers fills this gap by showing and analyzing the first rigorously evaluated global climatology of N_i, leading to new information shedding light on the processes that control high clouds.

Trends in China’s anthropogenic emissions since 2010 as the consequence of clean air actions

To tackle the problem of severe air pollution, China has implemented active clean air policies in recent years. We quantified China’s anthropogenic emissions during 2010–2017 and identified the major driving forces of these trends by using a combination of bottom-up emission inventory and index decomposition analysis (IDA) approaches. The major air pollutants have reduced their emissions by 17–62 % during 2010–2017. The IDA results suggest that emission control measures are the main drivers.

How well do stratospheric reanalyses reproduce high-resolution satellite temperature measurements?

Reanalyses (RAs) are models which assimilate observations and are widely used as proxies for the true atmospheric state. Here, we resample six leading RAs using the weighting functions of four high-res satellite instruments, allowing a like-for-like comparison. We find that the RAs generally reproduce the satellite data well, except at high altitudes and in the tropics. However, we also find that the RAs more tightly correlate with each other than with observations, even those they assimilate.

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