The global importance of gas-phase peroxy radical accretion reactions for secondary organic aerosol loading Atmospheric Chemistry and Physics DOI 10.5194/acp-25-17027-2025 28 November 2025 This work outlines an investigation into an understudied atmospheric chemical reaction pathway with the potential to form particulate pollution that has important impacts on air quality and climate. It suggests that this chemical pathway is responsible for a large fraction of the atmospheric particulate matter observed in tropical forested regions, but also highlights the need for further ambient and lab investigations to inform an accurate representation of this process in atmospheric models. Read more
Conflict-induced ship traffic disruptions constrain cloud sensitivity to stricter marine pollution regulations Atmospheric Chemistry and Physics DOI 10.5194/acp-25-16401-2025 21 November 2025 Militia attacks on ships in the Red Sea disrupted container ship traffic in 2024. We use these traffic changes to quantify how the cloud-altering properties of ship pollution decreased following sulfur regulations in 2020 with measurements of two types of ship pollution, one of which is sensitive to fuel composition and another which is not. Near Africa, cloud changes in 2024 were nearly as large as before the regulations, but only one-third as strong after accounting for increased traffic. Read more
The frosty frontier: redefining the mid-latitude tropopause using the relative humidity over ice Atmospheric Chemistry and Physics DOI 10.5194/acp-25-16303-2025 19 November 2025 We present a new technique to determine the tropopause based on the gradient of relative humidity over ice. This approach captures the character of the tropopause remarkably well, both in individual vertical profiles and in long-term averages, providing a consistent and physically meaningful representation of the transition between the troposphere and the stratosphere. Read more
Observed and modeled Arctic airmass transformations during warm air intrusions and cold air outbreaks Atmospheric Chemistry and Physics DOI 10.5194/acp-25-15047-2025 7 November 2025 Aircraft observations of air parcels moving into and out of the Arctic are reported. From the data, heating and cooling as well as drying and moistening of the air masses along their way into and out of the Arctic could be measured for the first time. These data are used to evaluate if weather prediction models are able to accurately represent these air mass transformations. This work helps to model the future Arctic climate changes, which may have an impact for mid-latitude weather as well. Read more
Review of interactive open-access publishing with community-based open peer review for improved scientific discourse and quality assurance Atmospheric Chemistry and Physics DOI 10.5194/acp-25-13903-2025 28 October 2025 Over 25 years, the European Geosciences Union (EGU) has demonstrated the success, viability and benefits of interactive open-access (OA) publishing with public peer review in its journals, its publishing platform EGUsphere and virtual compilations. The article summarizes the evolution of the EGU/Copernicus publications and of OA publishing with interactive public peer review at large by placing the EGU/Copernicus publications in the context of current and future global open science. Read more
The role of the tropical carbon balance in determining the large atmospheric CO2 growth rate in 2023 Atmospheric Chemistry and Physics DOI 10.5194/acp-25-13053-2025 25 October 2025 The year 2023 saw unexpectedly large global atmospheric CO2 growth. Satellite data reveal a role for increased tropical emissions. Larger emissions over eastern Brazil can be explained by warmer temperatures, which has led to exceptional drought, while hydrological changes play more of a role in emission increases elsewhere in the tropics. Broadly, we find that this situation continues into 2024. Read more
MOSAiC studies of long-lasting mixed-phase cloud events and analysis of the liquid-phase properties of Arctic clouds Atmospheric Chemistry and Physics DOI 10.5194/acp-25-12955-2025 21 October 2025 We studied the water and ice phases of Arctic mixed-phase clouds (MPCs) using dual FOV polarization lidar and Doppler radar on board Polarstern during the MOSAiC expedition. Two long-lasting Arctic MPCs and year-round statistics show persistent droplet activation and dominant immersion freezing, indicating well-filled cloud condensation nuclei and ice-nucleating particle reservoirs. These findings help explain MPC longevity and may improve cloud life cycle representation in weather and climate models. Read more
Light scattering and microphysical properties of atmospheric bullet rosette ice crystals Atmospheric Chemistry and Physics DOI 10.5194/acp-25-8785-2025 14 August 2025 Understanding the interaction between cirrus clouds and solar radiation is critical for modeling the Earth’s climate. A common crystal type found in cirrus clouds is the bullet rosette. Here, atmospheric bullet rosettes measured from jet aircraft are analyzed for their morphological and radiative properties. Atmospheric bullet rosettes are found to be more morphologically complex than previously assumed. This complexity has a significant impact on their radiative properties. Read more
Opinion: The role of AerChemMIP in advancing climate and air quality research Atmospheric Chemistry and Physics DOI 10.5194/acp-25-8289-2025 31 July 2025 The Aerosol Chemistry Model Intercomparison Project (AerChemMIP) aimed to quantify the climate and air quality impacts of aerosols and chemically reactive gases. We review its contribution to AR6 (Sixth Assessment Report of the Intergovernmental Panel on Climate Change) and the wider understanding of the role of these species in climate and climate change. We identify challenges and provide recommendations to improve the utility and uptake of climate model data, detailed summary tables of CMIP6 models, experiments, and emergent diagnostics. Read more
Observational constraints suggest a smaller effective radiative forcing from aerosol–cloud interactions Atmospheric Chemistry and Physics DOI 10.5194/acp-25-7299-2025 17 July 2025 This study addresses the long-standing challenge of quantifying the impact of aerosol–cloud interactions. Using satellite observations, reanalysis data, and a “perfect-model” cross-validation, we show that explicitly accounting for aerosol–cloud droplet activation rates is key to accurately estimating ERFaci (effective radiative forcing due to aerosol–cloud interactions). Our results indicate a smaller and less uncertain ERFaci than previously assessed, implying the reduced role of aerosol–cloud interactions in shaping climate sensitivity. Read more