The role of meteorological conditions and pollution control strategies in reducing air pollution in Beijing during APEC 2014 and Victory Parade 2015 Atmospheric Chemistry and Physics DOI 10.5194/acp-17-13921-2017 23 November 2017 The generalized linear regression model (GLM), even based only on meteorological parameters, could be satisfactory to estimate the contribution of meteorological conditions in reducing air pollution and hence the contribution of control strategies in reducing air pollution. Using the GLM, we found that the meteorological conditions and pollution control strategies contributed 30% and 28% to the reduction of the PM2.5 concentration during APEC 2014 and 38% and 25% during Parade 2015. APEC 2014 and Victory Parade 2015">Read more
A new diagnostic for tropospheric ozone production Atmospheric Chemistry and Physics DOI 10.5194/acp-17-13669-2017 17 November 2017 Understanding tropospheric ozone chemistry has been at the centre of the field of atmospheric chemistry for the last 30 years. However, our conceptual approach to diagnosing ozone production in global models has not advanced in this time. Our work presents a new and powerful approach for diagnosing tropospheric ozone production, providing a significant enhancement in our ability to understand the processes controlling ozone and how we can validate our assessment of these processes. Read more
Impact of agricultural emission reductions on fine-particulate matter and public health Atmospheric Chemistry and Physics DOI 10.5194/acp-17-12813-2017 27 October 2017 This study shows that agricultural emissions are important for air quality and their reduction can effectively reduce the concentration of fine particles and their associated premature mortality. Therefore, emission control policies, especially in North America and Europe, should also involve strong ammonia emission decreases to optimally reduce fine-particle concentration. Read more
A growing threat to the ozone layer from short-lived anthropogenic chlorocarbons Atmospheric Chemistry and Physics DOI 10.5194/acp-17-11929-2017 12 October 2017 We have observed large amounts of man-made chlorine compounds in E and SE Asia and in the upper tropical troposphere. These relatively short-lived compounds are not controlled by the Montreal Protocol, but if significant quantities were able to reach the stratosphere, the long-term recovery of stratospheric ozone would be delayed. We have also identified an important atmospheric transport mechanism that can rapidly transport these chemicals from E Asia to the upper troposphere via the tropics. Read more
An update on ozone profile trends for the period 2000 to 2016 Atmospheric Chemistry and Physics DOI 10.5194/acp-17-10675-2017 11 September 2017 Thanks to the 1987 Montreal Protocol and its amendments, ozone-depleting chlorine (and bromine) in the stratosphere has declined slowly since the late 1990s. Improved and extended long-term ozone profile observations from satellites and ground-based stations confirm that ozone is responding as expected and has increased by about 2 % per decade since 2000 in the upper stratosphere, around 40 km altitude. At lower altitudes, however, ozone has not changed significantly since 2000. Read more
Simultaneous measurements of new particle formation at 1 s time resolution at a street site and a rooftop site Atmospheric Chemistry and Physics DOI 10.5194/acp-17-9469-2017 8 August 2017 This study reports the distinct effects of street canyons on new particle formation (NPF) under warm or cold ambient temperature conditions because of on-road vehicle emissions; i.e., stronger condensation sinks are responsible for the reduced NPF in the springtime, but efficient nucleation and partitioning of gaseous species contribute to the enhanced NPF in the wintertime. The oxidization of biogenic organics is suggested to play an important role in growing new particles. Read more
NOx emission trends over Chinese cities estimated from OMI observations during 2005 to 2015 Atmospheric Chemistry and Physics DOI 10.5194/acp-17-9261-2017 1 August 2017 We assess NOx emission trends over Chinese cities based on satellite NO2 observations using a method independent of chemical transport models. NOx emissions over 48 Chinese cities have decreased significantly since 2011. Cities with different dominant emission sources (i.e. power, industrial, and transportation sectors) showed variable emission decline timelines that corresponded to the schedules for emission control in different sectors. OMI observations during 2005 to 2015">Read more
Exploring gravity wave characteristics in 3-D using a novel S-transform technique: AIRS/Aqua measurements over the Southern Andes and Drake Passage Atmospheric Chemistry and Physics DOI 10.5194/acp-17-8553-2017 13 July 2017 We introduce a novel 3-D method of measuring atmospheric gravity waves, based around a 3-D Stockwell transform. Our method lets us measure new properties, including wave intrinsic frequencies and phase and group velocities. We apply it to data from the AIRS satellite instrument over the Southern Andes for two consecutive winters. Our results show clear evidence that the waves measured are primarily orographic in origin, and that their group velocity vectors are focused into the polar night jet. AIRS/Aqua measurements over the Southern Andes and Drake Passage">Read more
Detectability of Arctic methane sources at six sites performing continuous atmospheric measurements Atmospheric Chemistry and Physics DOI 10.5194/acp-17-8371-2017 11 July 2017 Atmospheric methane simulations in the Arctic have been made for 2012 and compared to continuous observations at six measurement sites. All methane sources significantly affect the measurements at all stations, at least at the synoptic scale, except for biomass burning. An appropriate modelling framework combined with continuous observations of atmospheric methane enables us to gain knowledge on regional methane sources, including those which are usually poorly represented, such as freshwater. Read more
Opposite long-term trends in aerosols between low and high altitudes: a testimony to the aerosol–PBL feedback Atmospheric Chemistry and Physics DOI 10.5194/acp-17-7997-2017 30 June 2017 Opposite trends in aerosol loading between the lower and upper planetary boundary layer are found on a wide range of timescales and from different types of data acquired by various platforms in China. The reversal trend is consistent with the strong vertical gradients in the aerosol-induced atmospheric heating rate that unevenly modifies the atmospheric temperature profile and alters the stability differently. The findings have multiple implications in understanding and combating air pollution. Read more