Future air quality in Europe: a multi-model assessment of projected exposure to ozone Atmospheric Chemistry and Physics DOI 10.5194/acp-12-10613-2012 13 November 2012 In order to explore future air quality in Europe at the 2030 horizon, two emission scenarios developed in the framework of the Global Energy Assessment including varying assumptions on climate and energy access policies are investigated with an ensemble of six regional and global atmospheric chemistry transport models. Read more
Multi-generation gas-phase oxidation, equilibrium partitioning, and the formation and evolution of secondary organic aerosol Atmospheric Chemistry and Physics DOI 10.5194/acp-12-9505-2012 22 October 2012 A new model of secondary organic aerosol (SOA) formation is developed that explicitly takes into account multi-generational oxidation as well as fragmentation of gas-phase compounds, and assumes equilibrium gas-particle partitioning. Read more
Contrasting trends of mass and optical properties of aerosols over the Northern Hemisphere from 1992 to 2011 Atmospheric Chemistry and Physics DOI 10.5194/acp-12-9387-2012 15 October 2012 This study compares the long-term variation of mass and optical properties of atmospheric aerosols over the Northern Hemisphere, including China, the US, Canada and Europe. Contrasting trends of mass and optical properties were found from 1992 to 2011. Read more
Particle backscatter and relative humidity measured across cirrus clouds and comparison with microphysical cirrus modelling Atmospheric Chemistry and Physics DOI 10.5194/acp-12-9135-2012 5 October 2012 Advanced measurement and modelling techniques are employed to estimate the partitioning of atmospheric water between the gas phase and the condensed phase in and around cirrus clouds, and thus to identify in-cloud and out-of-cloud supersaturations with respect to ice. Read more
Diurnal variations of organic molecular tracers and stable carbon isotopic composition in atmospheric aerosols over Mt. Tai in the North China Plain: an influence of biomass burning Atmospheric Chemistry and Physics DOI 10.5194/acp-12-8359-2012 18 September 2012 This study demonstrates that crop-residue burning activities can significantly enhance the organic aerosol loading and alter the organic composition and stable carbon isotopic composition of aerosol particles in the troposphere over the North China Plain. Read more
Occurrence of lower cloud albedo in ship tracks Atmospheric Chemistry and Physics DOI 10.5194/acp-12-8223-2012 12 September 2012 The concept of geoengineering by marine cloud brightening is based on seeding marine stratocumulus clouds with sub-micrometer sea-salt particles to enhance the cloud droplet number concentration and cloud albedo, thereby producing a climate cooling effect. The efficacy of this as a strategy for global cooling rests on the extent to which aerosol-perturbed marine clouds will respond with increased albedo. It is found that the sign (increase or decrease) and magnitude of the albedo response in ship tracks depends on the mesoscale cloud structure, the free tropospheric humidity, and cloud top height. Read more
Summer ammonia measurements in a densely populated Mediterranean city Atmospheric Chemistry and Physics DOI 10.5194/acp-12-7557-2012 20 August 2012 Real-time measurements of ambient concentrations of gas-phase ammonia (NH3) were performed in Barcelona (NE Spain) in summer between May and September 2011. Two measurement sites were selected: one in an urban background traffic-influenced area (UB) and the other in the historical city centre (CC). Read more
Effects of business-as-usual anthropogenic emissions on air quality Atmospheric Chemistry and Physics DOI 10.5194/acp-12-6915-2012 1 August 2012 The atmospheric chemistry general circulation model EMAC has been used to estimate the impact of anthropogenic emission changes on global and regional air quality in recent and future years (2005, 2010, 2025 and 2050). The emission scenario assumes that population and economic growth largely determine energy and food consumption and consequent pollution sources with the current technologies (“business as usual”). Read more
Introduction to the European Monitoring and Evaluation Programme (EMEP) and observed atmospheric composition change during 1972–2009 Atmospheric Chemistry and Physics DOI 10.5194/acp-12-5447-2012 22 June 2012 European scale harmonized monitoring of atmospheric composition was initiated in the early 1970s, and the activity has generated a comprehensive dataset which allows the evaluation of regional and spatial trends of air pollution during a period of nearly 40 yr. EMEP) and observed atmospheric composition change during 1972–2009">Read more
Estimating the climate significance of halogen-driven ozone loss in the tropical marine troposphere Atmospheric Chemistry and Physics DOI 10.5194/acp-12-3939-2012 4 May 2012 We find that the implementation of oceanic halogen sources and chemistry in climate models is an important component of the natural background ozone budget and we suggest that it needs to be considered when estimating both preindustrial ozone baseline levels and long term changes in tropospheric ozone. Read more
