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Evaluating the PurpleAir monitor as an aerosol light scattering instrument

We show that the low-cost PurpleAir sensor can be characterized as a cell-reciprocal nephelometer. At two very different locations (Mauna Loa Observatory in Hawaii and the Table Mountain rural site in Colorado), the PurpleAir measurements are highly correlated with the submicrometer aerosol scattering coefficient measured by a research-grade integrating nephelometer. These results imply that, with care, PurpleAir data may be used to evaluate climate and air quality models.

The ESA MIPAS/Envisat level2-v8 dataset: 10 years of measurements retrieved with ORM v8.22

The level-2 v8 database from the measurements of the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS), aboard the European Space Agency Envisat satellite, containing atmospheric fields of pressure, temperature, and volume mixing ratio of 21 trace gases, is described in this paper. The database covers all the measurements acquired by MIPAS (from July 2002 to April 2012). The number of species included makes it of particular importance for the studies of stratospheric chemistry.

ESA MIPAS/Envisat level2-v8 dataset: 10 years of measurements retrieved with ORM v8.22">Read more

Options to correct local turbulent flux measurements for large-scale fluxes using an approach based on large-eddy simulation

Turbulent flux measurements suffer from a general systematic underestimation. One reason for this bias is non-local transport by large-scale circulations. A recently developed model for this additional transport of sensible and latent energy is evaluated for three different test sites. Different options on how to apply this correction are presented, and the results are evaluated against independent measurements.

Tracking aerosols and SO2 clouds from the Raikoke eruption: 3D view from satellite observations

The 21 June 2019 eruption of the Raikoke volcano produced significant amounts of volcanic aerosols (sulfate and ash) and sulfur dioxide (SO2) gas that penetrated into the lower stratosphere. We showed that the amount of SO2 decreases with a characteristic period of 8–18 d and the peak of sulfate aerosol lags the initial peak of SO2 by 1.5 months. We also examined the dynamics of an unusual stratospheric coherent circular cloud of SO2 and aerosol observed from 18 July to 22 September 2019.

A differential emissivity imaging technique for measuring hydrometeor mass and type

This paper describes a new instrument for quantifying the physical characteristics of hydrometeors such as snow and rain. The device can measure the mass, size, density and type of individual hydrometeors as well as their bulk properties. The instrument is called the Differential Emissivity Imaging Disdrometer (DEID) and is composed of a thermal camera and hotplate. The DEID measures hydrometeors at sampling frequencies up to 1 Hz with masses and effective diameters greater than 1 µg and 200 µm.

Rapid measurement of RH-dependent aerosol hygroscopic growth using a humidity-controlled fast integrated mobility spectrometer (HFIMS)

In this study, we present a newly developed instrument, the humidity-controlled fast integrated mobility spectrometer (HFIMS), for fast measurements of aerosol hygroscopic growth. The HFIMS can measure the distributions of particle hygroscopic growth factors at six diameters from 35 to 265 nm under five RH levels from 20 to 85 % within 25 min. The HFIMS significantly advances our capability of characterizing the hygroscopic growth of atmospheric aerosols over a wide range of relative humidities.

HFIMS)">Read more

The nano-scanning electrical mobility spectrometer (nSEMS) and its application to size distribution measurements of 1.5–25 nm particles

We present the design, modeling, and experimental characterization of the nano-scanning electrical mobility spectrometer (nSEMS), a recently developed instrument that probes particle physical properties in the 1.5–25 nm range. The nSEMS has proven to be extremely powerful in examining atmospheric nucleation and the subsequent growth of nanoparticles in the CERN CLOUD experiment, which provides a valuable asset to study atmospheric nanoparticles and to evaluate their impact on climate.

Physical characteristics of frozen hydrometeors inferred with parameter estimation

Satellite observations sensitive to cloud and precipitation help improve the quality of weather forecasts. However, they are sensitive to things that models do not forecast, such as the shapes and sizes of snow and ice particles. These details can be estimated from the observations themselves and then incorporated in the satellite simulators used in weather forecasting. This approach, known as parameter estimation, will be increasingly useful to build models of poorly known physical processes.

Iodide CIMS and m∕z 62: the detection of HNO3 as NO3− in the presence of PAN, peroxyacetic acid and ozone

We demonstrate in laboratory experiments that the formation of IOx anions (formed in reactions of I− with O3) or acetate anions (formed e.g. by the reaction of I− with peracetic acid) results in unexpected sensitivity of an iodide chemical ionisation mass spectrometer (I-CIMS) to HNO3 at a mass-to-charge ratio of 62. This helps explain observations of apparent high daytime levels of N2O5. Airborne measurements using I-CIMS confirm these conclusions.

CIMS and m∕z 62: the detection of HNO3 as NO3− in the presence of PAN, peroxyacetic acid and ozone">Read more

Characterization of dark current signal measurements of the ACCDs used on board the Aeolus satellite

This paper reports on dark current signal anomalies of the detectors used on board the ESA’s Earth Explorer satellite Aeolus during the first 1.5 years in orbit. After introducing sophisticated algorithms to classify dark current anomalies according to their characteristics, the impact of the different kinds of anomalies on wind measurements is discussed. In addition, mitigation approaches for the wind retrieval are presented and potential root causes are discussed.

ACCDs used on board the Aeolus satellite">Read more

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