Global distribution of methane emissions, emission trends, and OH concentrations and trends inferred from an inversion of GOSAT satellite data for 2010–2015 Atmospheric Chemistry and Physics DOI 10.5194/acp-19-7859-2019 12 June 2019 We use 2010–2015 satellite observations of atmospheric methane to improve estimates of methane emissions and their trends, as well as the concentration and trend of tropospheric OH (hydroxyl radical, methane’s main sink). We find overestimates of Chinese coal and Middle East oil/gas emissions in the prior estimate. The 2010–2015 growth in methane is attributed to an increase in emissions from India, China, and areas with large tropical wetlands. The contribution from OH is small in comparison. Read more
High-frequency monitoring of anomalous methane point sources with multispectral Sentinel-2 satellite observations Atmospheric Measurement Techniques DOI 10.5194/amt-14-2771-2021 31 May 2021 Satellites can detect methane emissions by measuring sunlight reflected from the Earth’s surface and atmosphere. Here we show that the European Space Agency’s Sentinel-2 twin satellites can be used to monitor anomalously large methane point sources around the world, with global coverage every 2–5 days and 20 m spatial resolution. We demonstrate this previously unreported capability through high-frequency Sentinel-2 monitoring of two strong methane point sources in Algeria and Turkmenistan. Read more
Ideas and perspectives: Sea-level change, anaerobic methane oxidation, and the glacial–interglacial phosphorus cycle Biogeosciences DOI 10.5194/bg-19-1421-2022 30 May 2022 A glacial–interglacial methane-fuelled redistribution of reactive phosphorus between the oceanic and sedimentary phosphorus reservoirs can occur in the ocean when falling sea level lowers the pressure on the seafloor, destabilizes methane hydrates, and triggers the dissolution of P-bearing iron oxides. The mass of phosphate potentially mobilizable from the sediment is similar to the size of the current oceanic reservoir. Hence, this process may play a major role in the marine phosphorus cycle. Read more
High-resolution underwater laser spectrometer sensing provides new insights into methane distribution at an Arctic seepage site Ocean Science DOI 10.5194/os-15-1055-2019 13 August 2019 Methane seepage from the seafloor west of Svalbard was investigated with a fast-response membrane inlet laser spectrometer. The acquired data were in good agreement with traditional sparse discrete water sampling, subsequent gas chromatography, and with a new 2-D model based on echo-sounder data. However, the acquired high-resolution data revealed unprecedented details of the methane distribution, which highlights the need for high-resolution measurements for future climate studies. Read more
Ideas and perspectives: is shale gas a major driver of recent increase in global atmospheric methane? Biogeosciences DOI 10.5194/bg-16-3033-2019 14 August 2019 Atmospheric methane has risen rapidly since 2008 and has become more depleted in 13C, in contrast to the trend towards more 13C enrichment in the late 20th century. Many have used this isotopic evidence to infer an increased biogenic source. Here I analyze the 13C trend with the consideration that methane from shale gas is somewhat depleted in 13C compared to other fossil fuels. I conclude that shale gas may be responsible for a third of the global increase from all sources. Read more
Methane emissions from the Munich Oktoberfest Atmospheric Chemistry and Physics DOI 10.5194/acp-20-3683-2020 3 April 2020 We demonstrate for the first time that large festivals can be significant methane sources, though they are not included in emission inventories. We combined in situ measurements with a Gaussian plume model to determine the Oktoberfest emissions and show that they are not due solely to human biogenic emissions, but are instead primarily fossil fuel related. Our study provides the foundation to develop reduction policies for such events and new pathways to mitigate fossil fuel methane emissions. Read more
Continuous weekly monitoring of methane emissions from the Permian Basin by inversion of TROPOMI satellite observations Atmospheric Chemistry and Physics DOI 10.5194/acp-23-7503-2023 28 July 2023 We use TROPOMI satellite observations to quantify weekly methane emissions from the US Permian oil and gas basin from May 2018 to October 2020. We find that Permian emissions are highly variable, with diverse economic and activity drivers. The most important drivers during our study period were new well development and natural gas price. Permian methane intensity averaged 4.6% and decreased by 1% per year. Read more
High-resolution interpolar difference of atmospheric methane around the Last Glacial Maximum Biogeosciences DOI 10.5194/bg-9-3961-2012 16 October 2012 Here we present new high-resolution methane records from the North Greenland Ice Core Project and the European Project for Ice Coring in Antarctica Dronning Maud Land ice cores covering Termination 1, the Last Glacial Maximum, and parts of the last glacial back to 32 000 years before present. Read more
High spatial resolution imaging of methane and other trace gases with the airborne Hyperspectral Thermal Emission Spectrometer (HyTES) Atmospheric Measurement Techniques DOI 10.5194/amt-9-2393-2016 1 June 2016 Using data from a new airborne Hyperspectral Thermal Emission Spectrometer (HyTES) instrument, we present a technique for the detection and wide-area mapping of emission plumes of methane and other atmospheric trace gas species over challenging and diverse environmental conditions with high spatial resolution, that permits direct attribution to sources in complex environments. Read more
Methanesulfonic acid (MSA) migration in polar ice: data synthesis and theory The Cryosphere DOI 10.5194/tc-11-2439-2017 3 November 2017 We combine a synthesis of 22 ice core records and a model of soluble impurity transport to investigate the enigmatic, post-depositional migration of methanesulfonic acid in polar ice. Our findings suggest that migration may be universal across coastal regions of Greenland and Antarctica, though it is mitigated at sites with higher accumulation and (or) lower impurity content. Records exhibiting severe migration may still be useful for inferring decadal and lower-frequency climate variability. Read more