Long-term historical trends in air pollutant emissions in Asia: Regional Emission inventory in ASia (REAS) version 3 Atmospheric Chemistry and Physics DOI 10.5194/acp-20-12761-2020 4 December 2020 A long historical emission inventory of major air pollutants in Asia during 1950–2015 was developed as Regional Emission inventory in ASia version 3 (REASv3). Trends of emissions and changes in source contributions in countries and regions in Asia during these 6 decades were analyzed. REASv3 provides monthly gridded data with 0.25° by 0.25° resolution for major source categories as well as table of emissions by countries and sub-regions for major sectors and fuel types. Read more
The Pliocene Model Intercomparison Project Phase 2: large-scale climate features and climate sensitivity Climate of the Past DOI 10.5194/cp-16-2095-2020 3 December 2020 The large-scale features of middle Pliocene climate from the 16 models of PlioMIP Phase 2 are presented. The PlioMIP2 ensemble average was ~ 3.2 °C warmer and experienced ~ 7 % more precipitation than the pre-industrial era, although there are large regional variations. PlioMIP2 broadly agrees with a new proxy dataset of Pliocene sea surface temperatures. Combining PlioMIP2 and proxy data suggests that a doubling of atmospheric CO 2 would increase globally averaged temperature by 2.6–4.8 °C. Read more
Vertical variability of the properties of highly aged biomass burning aerosol transported over the southeast Atlantic during CLARIFY-2017 Atmospheric Chemistry and Physics DOI 10.5194/acp-20-12697-2020 2 December 2020 Airborne measurements of highly aged biomass burning aerosols (BBAs) over the remote southeast Atlantic provide unique aerosol parameters for climate models. Our observations demonstrate the persistence of strongly absorbing BBAs across wide regions of the South Atlantic. We also found significant vertical variation in the single-scattering albedo of these BBAs, as a function of relative chemical composition and size. Aerosol properties in the marine BL are suggested to be separated from the FT. Read more
A microphysics guide to cirrus – Part 2:Climatologies of clouds and humidity from observations Atmospheric Chemistry and Physics DOI 10.5194/acp-20-12569-2020 1 December 2020 To improve the representations of cirrus clouds in climate predictions, extended knowledge of their properties and geographical distribution is required. This study presents extensive airborne in situ and satellite remote sensing climatologies of cirrus and humidity, which serve as a guide to cirrus clouds. Further, exemplary radiative characteristics of cirrus types and also in situ observations of tropical tropopause layer cirrus and humidity in the Asian monsoon anticyclone are shown. Read more
The Aarhus Chamber Campaign on Highly Oxygenated Organic Molecules andAerosols (ACCHA): particle formation, organic acids, and dimer esters fromα-pinene ozonolysis at different temperatures Atmospheric Chemistry and Physics DOI 10.5194/acp-20-12549-2020 30 November 2020 Atmospheric particles are important in relation to human health and the global climate. As the global temperature changes, so may the atmospheric chemistry controlling the formation of particles from reactions of naturally emitted volatile organic compounds (VOCs). In the current work, we show how temperatures influence the formation and chemical composition of atmospheric particles from α-pinene: a biogenic VOC largely emitted in high-latitude environments such as the boreal forests. Read more
Large contribution of organics to condensational growth and formation of cloud condensation nuclei (CCN) in the remote marine boundary layer Atmospheric Chemistry and Physics DOI 10.5194/acp-20-12515-2020 27 November 2020 Condensational growth of Aitken-mode particles is a major source of cloud condensation nuclei in the remote marine boundary layer. It has been long thought that over remote oceans, condensation growth is dominated by sulfate that derives from ocean-emitted dimethyl sulfide. In this study, we present the first long-term observational evidence that, contrary to conventional thinking, organics play an even more important role than sulfate in particle growth over remote oceans throughout the year. Read more
Beaching patterns of plastic debris along the Indian Ocean rim Ocean Science DOI 10.5194/os-16-1317-2020 26 November 2020 A large percentage of global ocean plastic enters the Indian Ocean through rivers, but the fate of these plastics is generally unknown. In this paper, we use computer simulations to show that floating plastics beach and end up on coastlines throughout the Indian Ocean. Coastlines where a lot of plastic enters the ocean are heavily affected by beaching plastic, but plastics can also beach far from the source on remote islands and countries that contribute little plastic pollution of their own. Read more
Reviews and syntheses: The mechanisms underlying carbon storage in soil Biogeosciences DOI 10.5194/bg-17-5223-2020 25 November 2020 The 4 per 1000 initiative aims to restore carbon storage in soils to both mitigate climate change and contribute to food security. The French National Institute for Agricultural Research conducted a study to determine the carbon storage potential in French soils and associated costs. This paper is a part of that study. It reviews recent advances concerning the mechanisms that controls C stabilization in soils. Synthetic figures integrating new concepts should be of pedagogical interest. Read more
Global modeling of cloud water acidity, precipitation acidity, and acidinputs to ecosystems Atmospheric Chemistry and Physics DOI 10.5194/acp-20-12223-2020 24 November 2020 Cloud water pH affects atmospheric chemistry, and acid rain damages ecosystems. We use model simulations along with observations to present a global view of cloud water and precipitation pH. Sulfuric acid, nitric acid, and ammonia control the pH in the northern midlatitudes, but carboxylic acids and dust cations are important in the tropics and subtropics. The acid inputs to many nitrogen-saturated ecosystems are high enough to cause acidification, with ammonium as the main acidifying species. Read more
The Making of the New European Wind Atlas – Part 2: Production and evaluation Geoscientific Model Development DOI 10.5194/gmd-13-5079-2020 23 November 2020 This is the second of two papers that document the creation of the New European Wind Atlas (NEWA). The paper includes a detailed description of the technical and practical aspects that went into running the mesoscale simulations and the microscale downscaling for generating the climatology. A comprehensive evaluation of each component of the NEWA model chain is presented using observations from a large set of tall masts located all over Europe. Read more
A technical description of the Balloon Lidar Experiment (BOLIDE) Atmospheric Measurement Techniques DOI 10.5194/amt-13-5681-2020 19 November 2020 The Balloon Lidar Experiment was the first lidar dedicated to measurements in the mesosphere flown on a balloon. During a 6 d flight, it made high-resolution observations of polar mesospheric clouds which form at high latitudes during summer at ~ 83 km altitude and are the highest clouds in Earth’s atmosphere. We describe the instrument and assess its performance. We could detect fainter clouds with higher resolution than what is possible with ground-based instruments. Read more
Topographic controls on divide migration, stream capture, anddiversification in riverine life Earth Surface Dynamics DOI 10.5194/esurf-8-893-2020 18 November 2020 Organisms evolve in ever-changing environments under complex process interactions. We applied a new software modelling tool to assess how changes in river course impact the evolution of riverine species. Models illustrate the climatically and tectonically forced landscape changes that can drive riverine biodiversity, especially where topographic relief is low. This research demonstrates that river course changes can contribute to the high riverine biodiversity found in real-world lowland basins. Read more
Climate change as an incentive for future human migration Earth System Dynamics DOI 10.5194/esd-11-875-2020 17 November 2020 We examine the implications of future motivation for humans to migrate by analyzing today’s relationships between climatic factors and population density, with all other factors held constant. Such analyses are unlikely to make accurate predictions but can still be useful for informing discussions about the broad range of incentives that might influence migration decisions. Areas with the highest projected population growth rates tend to be the areas most adversely affected by climate change. Read more
Resolving multiple geological events using in situ Rb–Sr geochronology:implications for metallogenesis at Tropicana, Western Australia Geochronology DOI 10.5194/gchron-2-283-2020 17 November 2020 Using a relatively new dating technique, in situ Rb–Sr geochronology, we constrain the ages of two generations of mineral assemblages from the Tropicana Zone, Western Australia. The first, dated at ca. 2535 Ma, is associated with exhumation of an Archean craton margin and gold mineralization. The second, dated at ca. 1210 Ma, has not been previously documented in the Tropicana Zone. It is probably associated with Stage II of the Albany–Fraser Orogeny and additional gold mineralization. Read more
A feasibility study to use machine learning as an inversion algorithm for aerosol profile and property retrieval from multi-axis differentialabsorption spectroscopy measurements Atmospheric Measurement Techniques DOI 10.5194/amt-13-5537-2020 12 November 2020 This paper is about a feasibility study of applying a machine learning technique to derive aerosol properties from a single MAX-DOAS sky scan, which detects sky-scattered UV–visible photons at multiple elevation angles. Evaluation of retrieved aerosol properties shows good performance of the ML algorithm, suggesting several advantages of a ML-based inversion algorithm such as fast data inversion, simple implementation and the ability to extract information not available using other algorithms. Read more
Connecting flow–topography interactions, vorticity balance, baroclinicinstability and transport in the Southern Ocean: the case of an idealizedstorm track Ocean Science DOI 10.5194/os-16-1207-2020 12 November 2020 The dynamical balance of the Antarctic Circumpolar Current and its implications on the functioning of the world ocean are not fully understood and poorly represented in global circulation models. In this study, the sensitivities of an idealized Southern Ocean (SO) storm track are explored with a set of eddy-rich numerical simulations. We show that the classical partition between barotropic and baroclinic modes is sensitive to current–topography interactions in the mesoscale range of 10–100 km. Read more
Ionic aluminium concentrations exceed thresholds for aquatic health in Nova Scotian rivers, even during conditions of high dissolved organic carbon and low flow Hydrology and Earth System Sciences DOI 10.5194/hess-24-4763-2020 10 November 2020 Wild salmon numbers in Nova Scotia, Canada, have been plummeting in recent decades. In 2014, we launched an ionic aluminium monitoring program in Nova Scotia to see if this toxic element was a threat to salmon populations. We found that all 10 monitored rivers had ionic aluminium concentrations that exceeded the threshold for aquatic health. Our results demonstrate that elevated aluminium still threatens aquatic ecosystems and that delays in recovery from acid rain remains a critical issue. Read more
Factors controlling plankton community production, export flux, and particulate matter stoichiometry in the coastal upwelling system off Peru Biogeosciences DOI 10.5194/bg-17-4831-2020 10 November 2020 The eastern boundary upwelling system off Peru is among Earth’s most productive ocean ecosystems, but the factors that control its functioning are poorly constrained. Here we used mesocosms, moored ~ 6 km offshore Peru, to investigate how processes in plankton communities drive key biogeochemical processes. We show that nutrient and light co-limitation keep productivity and export at a remarkably constant level while stoichiometry changes strongly with shifts in plankton community structure. Read more
Hydrology and water resources management in ancient India Hydrology and Earth System Sciences DOI 10.5194/hess-24-4691-2020 5 November 2020 Like in all ancient civilisations, the need to manage water propelled the growth of hydrological science in ancient India also. In this paper, we provide some fascinating glimpses into the hydrological, hydraulic, and related engineering knowledge that existed in ancient India, as discussed in contemporary literature and recent explorations and findings. Many interesting dimensions of early scientific endeavours emerge as we investigate deeper into ancient texts, including Indian mythology. Read more
Impacts of future land use and land cover change on mid-21st-century surface ozone air quality: distinguishing between the biogeophysical and biogeochemical effects Atmospheric Chemistry and Physics DOI 10.5194/acp-20-11349-2020 5 November 2020 We investigate the effects of future land use and land cover change (LULCC) on surface ozone air quality worldwide and find that LULCC can significantly influence ozone in North America and Europe via modifying surface energy balance, boundary-layer meteorology, and regional circulation. The strength of such “biogeophysical effects” of LULCC is strongly dependent on forest type and generally greater than the “biogeochemical effects” via changing deposition and emission fluxes alone. Read more